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Studies on coherent and incoherent spin dynamics that control the magnetic field effect on photogenerated radical pairs
Published in Molecular Physics, 2020
Tomoaki Miura
Alternatively, there is a great possibility that the molecular dynamics can be quantitatively probed by observing the decoherence processes of radical pairs. Such an approach would help understanding complicated electron transfer mechanisms in biological and artificial systems. In the future, the mechanism of avian magnetoreception would be clarified by studying controlling mechanisms of the spin decoherence in avian cryptochrome with detailed analysis of experimental MFE by MD-assisted spin dynamics simulations. In the case of electron−hole pairs in organic semiconductor thin films, diffusion modelling based on the microscopic structures of the disordered organic solids and its combination with spin dynamics simulations would clarify the molecular-level mechanisms of charge extinction (mainly recombination) from electrically and/or optically detected MFE. Such studies would offer important feedback to development and engineering of these future materials.